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With a single-electrode model, we investigated surface charge screening at anionic liquid-electrode interface. Using the obtained geometric packingdensities, we estimated structure-determined potentials and capacitance valuesfor 40 studied ions. By comparing the predictions with the empirical data, weshow that exact surface charge screening by a monolayer of counter-ions (aswell as crowding of ions) is improbable for common ions within theirelectrochemical stability window. We also predict that theoretically such ascreening state is possible for frisbee-shape ions.

Ionic liquid-electrode interface: classification of ions, saturation of layers, and structure-determined potentials