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Due to the importance of using supercapacitors in electronic storage devices,improving their efficiency is one of the topics that has attracted theattention of many researchers. Choosing the proper electrolyte forsupercapacitors is one of the most significant factors affecting theperformance of supercapacitors. In this paper, two classes of electrolytes,i.e. liquid electrolyte (ionic liquid electrolyte) and solid electrolyte(polymer electrolyte) are compared by molecular dynamics simulation. Weconsider the polymer electrolyte in linear and network configurations. Theresults show that although ionic liquid-based supercapacitors have a largerdifferential capacitance, since they have a smaller operation voltage, theamount of energy stored is less than polymer electrolyte-based supercapacitors.Also, our investigations indicate that polymer electrolyte-basedsupercapacitors have more mechanical stability. Therefore, they can beconsidered a very suitable alternative to liquid electrolyte-basedsupercapacitors that do not have known liquid electrolyte problems and displaybetter performance.

Performance investigation of supercapacitors with PEO-based gel polymer & ionic liquid electrolytes: Molecular Dynamics Simulation