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Ultrafast quantum dynamics relaxation of a photoexcited state in a stronglycorrelated spin crossover system LaCoO3 under a sudden perturbation isconsidered with the density matrix generalized master equation. Themagnetization and cobalt-oxygen bond length oscillations were found. Theevolution of the electronic band structure during relaxation is calculated inthe framework of the LDA+GTB method.

Light-induced ultrafast dynamics of spin crossovers in LaCoO3