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Graphite intercalation compounds (GICs) with the geometrical anisotropy andstrong electron-phonon coupling are in full swing and have shown their greatpotential for applications in nanodevices. I selected representative threeelements in actinide group with valence electron arrangement: Thorium (Th)([Rn]6d27s2), Uranium (U) ([Rn]5f36d17s2), Plutonium (Pu) ([Rn]5f67s2). Icalculated their phonon spectra and demonstrated the atomic-scalemicrostructure identification of actinide graphite intercalation compounds byangle-resolved polarized Raman spectroscopy.

Angle-resolved polarized Raman spectroscopy for distinguishing stage-I graphite intercalation compounds with Thorium, Uranium and Plutonium