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Dissociative electron attachment (DEA) to gas-phase carbonyl sulfide (OCS)has been studied diligently using the time-of-flight (TOF) basedstate-of-the-art velocity map imaging (VMI) technique. Three well-resolved DEAresonances are observed at 5.0, 6.5 and 10.0 eV incident electron energiesalong with a weak structure at 8.0 eV. The velocity slice images (VSI), Kineticenergy (KE) and angular distributions (AD) for the fragmented sulfur anions areobtained using the wedge slicing technique. The KE distributions for the sulfurnascent fragments reveal bi-modality with rovibrational signatures. The ADssubstantiate speed-dependent angular anisotropy demand the existence of partialcorrelations among three different point group symmetries, confirmed through anin-plane bending mode of vibration with the axial recoil breakdown. Theoreticalcalculations using R-matrix and density functional approaches strongly supportthe experimental observations.

Observation of rovibrationally coupled bi-modality and speed-dependent  orientation in DEA dynamics of OCS: reveals partial correlations among point  group symmetries