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Discovery of intrinsic two-dimensional (2D) magnetic materials is crucial forunderstanding the fundamentals of 2D magnetism and realizing next-generationmagnetoelectronic and magneto-optical devices. Although significant effortshave been devoted to identifying 2D magnetism by exfoliating bulk magneticlayered materials, seldom studies are performed to synthesize ultra-thinmagnetic materials directly for non-layered magnetic materials. Here, we reportthe successful synthesis of a new type of theoretically proposed 2D metallicferromagnet 1T FeS2, through the molten-salt-assisted chemical vapor deposition(CVD) method. The long-range 2D ferromagnetic order is confirmed by theobservation of a large anomalous Hall effect (AHE) and a hystereticmagnetoresistance. The experimentally detected out-of-plane ferromagneticordering is theoretically suported with Stoner criterion. Our findings open upnew possibilities to search novel 2D ferromagnets in non-layered compounds andrender opportunities for realizing realistic ultra-thin spintronic devices.

1T-FeS$_2$$:$ a new type of two-dimensional metallic ferromagnet