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High internal phase emulsions (HIPEs) are considered as an importantfunctional material and have been the focus of intense development effort, butit has not been possible to alter their fundamental attributes at either themicrocosmic or macroscopic level, which severely limits their practicalapplications in various areas. In this work, we report a general strategy forcreating complex HIPEs and we additionally show a route to forming HIPE filmsat liquid interfaces. Double HIPEs and Janus HIPEs are both realized for thefirst time. They feature complex microscopic patterns with a short-rangeanisotropy, and exhibit non-Newtonian pseudoplastic flow behavior. By takingadvantage of their response to a high-pH subphase, interfacial films can besuccessfully obtained, which are tunable in thickness and morphologies undercompression.

Complex High Internal-Phase Emulsions that can Form Interfacial Films with Tuneable Morphologies