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Insufficient availability of molten salt corrosion-resistant alloys severelylimits the fruition of a variety of promising molten salt technologies thatcould otherwise have significant societal impacts. To accelerate alloydevelopment for molten salt applications and develop fundamental understandingof corrosion in these environments, here we present an integrated approachusing a set of high-throughput alloy synthesis, corrosion testing, and modelingcoupled with automated characterization and machine learning. By using thisapproach, a broad range of Cr-Fe-Mn-Ni alloys were evaluated for theircorrosion resistances in molten salt simultaneously demonstrating thatcorrosion-resistant alloy development can be accelerated by thousands of times.Based on the obtained results, we unveiled a sacrificial mechanism in thecorrosion of Cr-Fe-Mn-Ni alloys in molten salts which can be applied to protectthe less unstable elements in the alloy from being depleted, and provided newinsights on the design of high-temperature molten salt corrosion-resistantalloys.

Accelerated Discovery of Molten Salt Corrosion-resistant Alloy by High-throughput Experimental and Modeling Methods Coupled to Data Analytics