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We put forward a novel, twofold scheme that enables at the same timeall-optical enantioselection and sorting of single multipolar chiralmicrospheres based on optical pulling forces exerted by two non-collinear,nonstructured, circularly-polarized light sources. Our chiral resolution methodcan be externally controlled by varying the angle between their incidentwavevectors, allowing for a fine-tuning of the range of chiral indices forenantioselection. Enantioselectivity is achieved by choosing angles such thatonly particles with the same handedness of the light sources are pulled. Thisproposal allows one to achieve all-optical sorting of chiral microspheres witharbitrarily small chiral parameters, thus outperforming current opticalmethods.

Enantioselection and chiral sorting of single microspheres using optical pulling forces