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As a complementary analysis tool to conventional high-field NMR, zero- toultralow-field (ZULF) NMR detects nuclear magnetization signals in thesub-microtesla regime. Spin-exchange relaxation-free (SERF) atomicmagnetometers provide a new generation of sensitive detector for ZULF NMR. Dueto the features such as low-cost, high-resolution and potability, ZULF NMR hasrecently attracted considerable attention in chemistry, biology, medicine, andtests of fundamental physics. This review describes the basic principles,methodology and recent experimental and theoretical development of ZULF NMR, aswell as its applications in spectroscopy, quantum control, imaging, NMR-basedquantum devices, and tests of fundamental physics. The future prospects of ZULFNMR are also discussed.

Zero- to ultralow-field nuclear magnetic resonance and its applications