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Our computer simulations have shown that the large-scale conformationaldynamics of a short oligomeric fragment of thermoresponsive polymers resemblethe mechanical movement of nonlinear bistable systems. The oligomersdemonstrate spontaneous vibrations and stochastic resonance activated by thethermal noise. We have observed reasonable shifts of the spontaneous vibrationsand stochastic resonance modes when attaching a molecular cargo to theoligomer. All these effects indicate that bistable oligomers may work asoperational units capable of detecting single molecules.

Detection of single molecules using stochastic resonance of bistable oligomers