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Metal halide perovskites single-crystalline thin films (SCTFs) have recentlyemerged as promising materials for the next generation of optoelectronicdevices due to their superior intrinsic properties. However, it is stillchallenging to transfer and integrate them with other functional materials forhybrid multilayer devices because of their substrate-dependent growth. Herein,a method that allows the SCTFs to be transferred with high quality ontoarbitrary substrates has been reported. By introducing hydrophobic treatment tothe growth substrates, the adhesion between SCTFs and growth substrates isreduced. Meanwhile, anti-solvent intercalation technique is used to peel offSCTFs from the growth substrates intactly. Finally, centimeter-scale perovskiteSCTF has been successfully transferred to target substrate. This work opens upa new route to transfer large-scale perovskite SCTFs, providing a platform towiden the applications of perovskite SCTFs in large-scale hybrid multilayeroptoelectronic devices.

Transfer of large-scale perovskite single-crystalline thin films onto arbitrary substrates