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The recent advent of cutting-edge experimental techniques allows for aprecise synthesis of monodisperse subnanometer metal clusters composed by justa few atoms, and opens new possibilities for subnanometer science. Thedecoration of titanium dioxide surfaces with the Ag$_{5}$ atomic clusterenables the stabilization of surface polarons. A new electron polarizationphenomenon accompanying surface polaron formation has thus been revealed.

A new generation of subnanometer-sized materials reveals a general surface polarons property