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Here, the possibility of the existence of nitro-graphene derivatives withundisturbed graphene backbone is considered. Based on the first-principlescalculation, it is shown that while NO$_2$ is unable to form a covalent bondwith bare graphene, it becomes possible in some structures of graphane,fluorographene, and graphene oxide. This paper presents, among others, ananalysis of the surrounding influence on the C-NO$_2$ bond strength. The authorbelieves, that potential prospects of these materials and discussion aboutpossible synthesizing routes may help further research on graphene-basedmaterials.

On the stability and existence of nitro-graphene, nitro-graphane, and nitro-graphene oxide