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An ab initio simulation of strong-field photodissociation of diatomicmolecules was developed, inspired by recent dissociation experiments of F2-.The transition between electronic states was modeled, including the laser pulseand transition dipole, and the angle between them. The initial conditions ofthe system were set to be thermal and to include different rovibrationalstates. Carefully designed absorbing boundary conditions were applied todescribe the boundary conditions of the experiment. We studied the influence offield intensity on the direction of the outcoming fragments andlaboratory-fixed axis, defined by the field polarization. At high intensities,the angular distribution became more peaked with a marginal influence onkinetic energy release.

Dissociation in strong field: a quantum analysis of the relation between angular momentum and angular distribution of fragments