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We demonstrate the capability of block-copolymer templating to tune therefractive indices of functional oxides over a broad range by structuringmaterials on the 20-1000 atoms scale, with simple one-pot synthesis. Thepresented method is then combined with genetic algorithm-based optimization toexplore its application for anti-reflection coating design. Merging thesetechniques allows for the realization of a minimal two-layer anti-reflectionstack for silicon with broadband reflectivity of just 3% from the nominal valueof 38%, over a 120{\deg} angular span, validated by fabrication followed byoptical measurements.

Continuously tuning the refractive indices by restructuring materials on the 20-1000 atoms scale: improving anti-reflection coating designs