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Exploration of rare-earth (RE)-based Kagome lattice magnets with spin-orbitalentangled jeff=1/2 moments will provide new platform for investigating theexotic magnetic phases. Here, we report a new family of RE3BWO9(RE=Pr,Nd,Gd-Ho) boratotungstates with magnetic RE3+ ions arranged on Kagomelattice, and perform its structure and magnetic characterizations. This serialcompounds crystallize in hexagonal coordinated structure with space group P63(No.173), where magnetic RE3+ ions have distorted Kagom\'e lattice connectionswithin the ab plane and stacked in a AB-type fashion along c axis. Theinterlayer RE-RE separation is comparable with that of intralayer distance,forming 3-dimensional (3D) exchange coupled magnetic framework of RE3+ ions.The magnetic susceptibility data of RE3BWO9 (RE=Pr, Nd, Gd-Ho) reveal dominantantiferromagnetic interactions between magnetic RE3+ ions, but without visiblemagnetic ordering down to 2 K. The magnetization analyses for different RE3+ions show diverse anisotropic behaviors, make RE3BWO9 as an appealingKagome-lattice antiferromagnet to explore exotic magnetic phases.

A new family of disorder-free Rare-Earth-based kagom\'e lattice magnets:  structure and magnetic characterizations of RE3BWO9 (RE=Pr, Nd, Gd-Ho)  Boratotungstates