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In this work, a novel electrospun conductive polymer nanocomposite made ofpolycaprolactone with an exohedral complex made of multiwalled carbon nanotubesand fullerene C60 was prepared and characterized. The preparation wasstraightforward and the complexes self-assembled within the nanocompositefibers. The nanocomposite showed electrical switching behavior due to chargeaccumulation of fullerene C60 upon electrical stimulation. Write-once read-manymemory devices were fabricated by electrospinning a nanocomposite with 0.8%wt.fullerene C60 onto interdigitated coplanar electrodes. The device retained theON state for more than 60 days and could be thermally reset, reprogrammed anderased with subsequent electrical and thermal cycling. Moreover, the electricalresistance of the device could be modulated by applying different programmingvoltage amplitudes and programming times, which revealed its adaptive behaviorand potential application to neuromorphic systems.

An electrospun Polymer Composite with Fullerene-Multiwalled Carbon Nanotube Exohedral Complexes can act as Memory Device