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Spin-entaglement has been proposed and extensively used in the case ofcorrelated triplet pairs which are intermediate states in singlet fissionprocess in select organic semiconductors. Here, we employ quantum processtomography of polarization entangled photon-pairs resonant with the excitedstate absorption of these states to investigate the nature of the inherentquantum correlations and to explore for an unambiguous proof for the existenceof exciton entanglement.

Quantum process tomography of entangled photons as a probe of intermediates of singlet fission in a tetracene derivative