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Microwave synthesis was optimized for preparing novel monoclinic Tin-dopedBarium Niobate ceramics (Ba1-xSnxNb2O6; x= 0.0, 0.01, 0.05, 0.1, 0.2, 0.3) BSN.The intensity of monoclinic phase formation was observed to decrease onincreasing tin as dopant indicating decreased crystallinity. Strainedcrystalline phase was observed in undoped sample that became severe on dopingtin. Monoclinic metal alloy Sn2O3 formation was confirmed on increasing tindoping beyond 5%. Electronic configuration of tin (II) oxide supports the localsite-wise monoclinic disorder in crystal structure due to sterically activelone pair. Such a disorder arranges increased number of degenerate energystates and reduce effective energy gap between conduction band minimum andvalence band maximum. All BSN compositions were investigated for monoclinicphase stabilization, ultra-violet absorption, dielectric response, raman modesand type of carrier concentration along with hall resistivity. All measurementspossessed inflexion corresponding to 5 atomic % tin doping indicatingsuccessful site substitution and estimated Sn2O3 metal formation beyond this.The values of reducing optical energy band gap, transparency to visiblespectrum and hall resistivity indicated utility of these materials as asubstitute transparent conducting oxide (TCO) for well-known indium tin oxide(ITO).

Microwave derived monoclinic Ba1-xSnxNb2O6 materials as an alternative of ITO