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We predict a new quantum electronic structure at the interface between twocondensed phases of noble-gas elements: solid neon and superfluid helium. Anexcess electron injected onto this interface self-confines its wavefunctioninto a nanometric dome structure whose size varies with pressure. A collectionof such electrons can form a classical Wigner crystal visualizable bymid-infrared photons. The ultralong spin-coherence time allows the electrons inthis system to serve as perfect quantum bits. They can be deterministicallyarranged on-chip at a spacing of several microns. Their spin states can becontrolled and readout by single-electron devices. This unique system offers anappealing new architecture for scalable quantum information processing.

Quantum Electronic Structure at the Interface of Solid Neon and Superfluid Helium