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The PTFE (Teflon) has been selected as the self-template structural materialin preparation of VO2 films using reactive magnetron sputtering systems andpost annealing progress. Spontaneous random nano-porous structures of VO2 filmsgrowing on quartz glasses have been deliberately established via bottom-upprocessing through this novel and facile approach. The nano-porous VO2 filmsexhibit an excellent optical performance based on localized surface plasmonresonance (LSPR), with ultrahigh luminous transmittance (Tlum) up to 78.0% andthe promoted solar modulation ability ({\Delta}Tsol) of 14.1%. Meanwhile, theingenious microstructure of film provides an antireflection function frommultiple perspectives in visible light, with the potential of the windshield onvehicles for smart solar modulation. The nano-porous films expand the practicalapplication of thermochromic VO2 to a fire-new field, breaking the opticalperformance envelope of single-layer dense VO2 film away, and offering auniversal method to prepare homogeneous nano-porous structures for thin films.

Sputtered Spontaneously Nano-porous VO2-based Films via PTFE  Self-Template: Localized Surface Plasmon Resonance Induced Robust Optical  Performance for Solar Glazing Application