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We have investigated the metamagnetic-like transition in the triple layerruthenate Sr4Ru3O10 by means of neutron diffraction from single crystals. Themagnetic structure of the compound appears to be determined in a complex way bythe two substructures of inequivalent ruthenium ions. At Tc=105K the system hasa sharp transition into a ferromagnetic state along the c-axis which is drivenby the ruthenium atoms in the central octahedra of the triple layers whereasthe substructure of the outer ruthenium atoms tend to align in the ab planeachieving an antiferromagnetic order at the metamagnetic transition T*~50K.Below T* the strong anisotropy along c prevails, the outer ruthenium tend toalign along the c-axis and the in-plane antiferromagnetic order disappears.This finding confirms the delicate balance between antiferro and ferromagneticcouplings in the (Sr,Ca)n+1RunO3n+1 family of compounds, and proves the layerdependence of the magnetic anisotropy in Sr4Ru3O10.

Layer dependent antiferromagnetism in the Sr4Ru3O10 ruthenate at the metamagnetic-like transition