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Two-dimensional charge carrier accumulation at oxide heterointerfacespresents a paradigm shift for oxide electronics. Like a capacitor, interfacialcharge buildup couples to an electric field across the dielectric medium. Toprevent the so-called polar catastrophe, several charge screening mechanismsemerge, including polar distortions and interfacial intermixing which reducethe sharpness of the interface. Here, we examine how atomic intermixing atoxide interfaces affect the balance between polar distortions and electricpotential across the dielectric medium. We find that intermixing moves the peakcharge distribution away from the oxide/oxide interface; thereby changing thedirection of polar distortions away from this boundary with minimal effect onthe electric field. This opposing electric field and polar distortions isequivalent to the transient phase transition tipping point observed in doublewell ferroelectrics; resulting in an anomalous dielectric response -- apossible signature of local negative differential capacitance, withimplications for designing dissipationless oxide electronics.

Anomalous dielectric response at intermixed oxide heterointerfaces