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Spinterface engineering has shown quite important roles in organicspintronics as it can improve spin injection or extraction. In this study,11,11,12,12-tetracyanonaptho-2,6-quinodimethane (TNAP) is introduced as aninterfacial layer for a prototype interface of Fe/TNAP. We report anelement-specific investigation of the electronic and magnetic structures ofFe/TNAP system by use of near edge X-Ray absorption fine structure (NEXAFS) andX-ray magnetic circular dichroism (XMCD). Strong hybridization between TNAP andFe and induced magnetization of N atoms in TNAP molecule are observed. XMCD sumrule analysis demonstrates that the adsorption of TNAP reduces the spin momentof Fe by 12%. In addition, induced magnetization in N K-edge of TNAP has alsobeen found with other commonly used ferromagnets in organic spintronics, suchas La0.7Sr0.3MnO3 and permalloy, which makes TNAP a very promising molecule forspinterface engineering in organic spintronics.

11,11,12,12-tetracyanonaphtho-2,6-quinodimethane in Contact with Ferromagnetic Electrodes for Organic Spintronics