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Using an effective genetic algorithm, we uncover the structure of ametastable Al41Sm5 phase that supplements its family sharing similarshort-range orders. The phase evolves upon heating an amorphous Al-9.7at.%Smribbon, produced by melt-spinning. The dynamical phase selection is discussedwith respect to the structural connections between the short-range packingmotifs in the amorphous precursor and those observed in the selected phases.The phase elucidated here is one of several newly discovered large-unit-cellphases found to form during devitrification from the glass in this binarysystem, further illustrating the power and efficiency of our approach, theimportant role of structural hierarchy in phase selection, and the richness ofthe metastable phase landscape accessible from the glassy structure.

Observation of Al41Sm5: new evidence for structural hierarchy in Al-Sm alloys