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Despite recent significant developments of Si composites, use of silicon withsignificance in the anodes for Li-ion batteries is still limited. In fact,nominal energy density is to be saturated around ~750 Wh/L regardless ofcell-types under the current material strategies. Use of Si-rich anode can pushthe limit; however, the prolonged irreversible Li consumption becomes moreprominent. We previously showed that repeating c-Li3.75(+{\delta})Siformation/decomposition, typically recognized to degrade the anodes, canimprove the irreversibility and accumulatively minimize the gross consumption.Utilizing the insights combined with prelithiation techniques, here we provideprototypic cell designs that can nonlinearly deplete the consumption.

Strategy to Nonlinearly Deplete Irreversible Li Consumption in Si-rich Li-Ion Batteries