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While experiments with one or two quantum emitters have become routine invarious laboratories, scalable platforms for efficient optical coupling of manyquantum systems remain elusive. To address this issue, we report on chip-basedsystems made of one-dimensional subwavelength dielectric waveguides(nanoguides) and polycyclic aromatic hydrocarbon molecules. After discussingthe design and fabrication requirements, we present data on coherent linear andnonlinear spectroscopy of single molecules coupled to a nanoguide mode. Ourresults show that external microelectrodes as well as optical beams can be usedto switch the propagation of light in a nanoguide via the Stark effect and anonlinear optical process, respectively. The presented nanoguide architecturepaves the way for the investigation of many-body phenomena and polaritonicstates and can be readily extended to more complex geometries for therealization of quantum integrated photonic circuits.

On-chip linear and nonlinear control of single molecules coupled to a nanoguide