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The technique is presented of restoring the electronic density of states ofthe valence band from data of X-ray photoelectron spectroscopy. The originalityof the technique consists in using a stochastic procedure to solve an integralequation relating the density of states and the experimental X-rayphotoelectron spectra. The results are presented for bulk sample of gold andnanoclusters of tantalum; the possibility of using the results to determine thedensity of states of low-dimensional structures, including ensembles of metalnanoclusters, is demonstrated.

Calculation of density of states of transition metals: from bulk sample to nanocluster