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The radical anion salt [Fe{HC(pz)3}2](TCNQ)3 demonstrating conductivity andspin-crossover transition (SCO) associated with Fe(II) complex cation subsystemhas been synthesized and structurally characterized. A pronounced change of thedc resistivity and a robust broadening of the EPR signal triggered by the SCOtransition are found. Enhanced EPR line broadening is interpreted in terms ofcross relaxation between the TCNQ and Fe(II) spin subsystems

The conducting spin-crossover compound combining Fe(II) cation complex with TCNQ in a fractional reduction state