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Tremendous enhancement of light-matter interaction in plasmon-excitedmolecular hybrid devices allows for non-linearities on the level of singleemitters and few photons. This promises a plethora of novel applications likesingle photon transistors. Nevertheless, building the components of suchdevices is technologically extremely challenging. We tackle this task bylithographically fabricating on-chip plasmonic waveguides, efficientlyconnected to far-field in- and out-coupling ports via low-loss dielectricwaveguides. Furthermore, a nano-assembling technology is developed, enablingthe controlled coupling of single organic emitters to the plasmonic waveguides.Dibenzoterrylene fluorescent molecules hosted in anthracene crystals areinvestigated for this purpose. Here we present all key-components andtechnologies for a plasmon-excited single molecule non-linear device.

Key components for nano-assembled plasmon-excited single molecule non-linear devices