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We present here an investigation of the magnetic ordering in the Mottinsulating oxyselenide materials Ln2O2Fe2OSe2 (Ln = Ce, Nd). Neutron powderdiffraction data are consistent with a non-collinear multi-k ordering on theiron sublattice structure and analysis indicates a reduced magnetic correlationlength perpendicular to the [Fe2O]2+ layers. The magnetic role of the Ln3+cations is investigated and Ce3+ moments are found to order for T < 16 K.

Structural and magnetic characterisation of iron oxyselenides Ce2O2Fe2OSe2 and Nd2O2Fe2OSe2