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A general discussion of the simulation procedure of the full susceptibilitytensor and isothermal magnetization pseudovector for compounds comprisingweakly-interacting magnetic centers is presented. A single-crystal-sample aswell as a powder-sample case are considered. The procedure is used to obtainexplicit expressions for the full susceptibility tensor for spins S=1, 3/2, 2,and 5/2 for non-vanishing rhombic local anisotropy and any form ofspectroscopic tensor.

Full susceptibility tensor for localized spin models with S=1, 3/2, 2, 5/2 and with rhombic anisotropy