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We present a neutron powder diffraction study of the monoclinic doubleperovskite systems Nd2NaB'O6 (B' = Ru, Os), with magnetic atoms occupying boththe A and B' sites. Our measurements reveal coupled spin ordering between theNd and B' atoms with magnetic transition temperatures of 14 K for Nd2NaRuO6 and16 K for Nd2NaOsO6. There is a Type I antiferromagnetic structure associatedwith the Ru and Os sublattices, with the ferromagnetic planes stacked along thec-axis and [110] direction respectively, while the Nd sublattices exhibitcomplex, canted antiferromagnetism with different spin arrangements in eachsystem.

Coupled Nd and B' spin ordering in the double perovskites Nd2NaB'O6 (B' = Ru, Os)