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The surface or contact potential at the water liquid-vapor interface isdiscussed in relation to determinations of absolute ion hydration free energiesand distributions of ions near the interface. It is shown that, rather than thesurface potential itself, the net electrostatic potential at the center of anuncharged solute can aid both in relating differences between tabulations ofhydration free energies and in explaining differing classical and quantumsurface potential estimates. Quantum mechanical results are consistent withconclusions from classical simulations that there is a net driving force thatenhances anion density at the surface relative to cations.

The influence of water interfacial potentials on ion hydration free energies and density profiles near the surface