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Magnetic Resonance Imaging has become nowadays an indispensable tool withapplications ranging from medicine to material science. However, so far thephysical limits of the maximum achievable experimental contrast were unknown.We introduce an approach based on principles of optimal control theory toexplore these physical limits, providing a benchmark for numerically optimizedrobust pulse sequences which can take into account experimental imperfections.This approach is demonstrated experimentally using a model system of twospatially separated liquids corresponding to blood in its oxygenated anddeoxygenated forms.

Exploring the physical limits of saturation contrast in Magnetic Resonance Imagign