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A series of MnO2 unique nanostructures were synthesized by a facilehydrothermal method with microwave-assisted procedures. A novel nanostructureformation mechanism has been proposed, that MnO6 octahedral nuclei andmolecular layers can be rearranged into different nanostructured morphologiesby restacking and splitting, and then clasping, which is associated with tunnelstructure phase transformation. Systematic macrostructure observations andmagnetic property measurements have been conducted on these nanostructures,which demonstrate that engineering layered structures has the potential tocreate many unique nanostructures and unusual physicochemical behaviours.

Architected Various MnO6 Octahedral Layers MnO2 Nanostructures