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Effects of the adsorption-desorption process on the immittance response of anelectrolytic cell are theoretically investigated in the framework of thediffusional Poisson-Nernst-Planck (PNP) continuum model, when the generationand recombination of ions is taken into account. The analysis is carried out bysearching solutions for the drift-diffusion equation coupled to the Poisson'sequation relating the effective electric field to the net charge density. Theeffect of different ion mobilities on the immittance, i.e., situations withequal and different diffusion coefficients for positive and negative ions, areconsidered. A general exact expression for the admittance in the context of thelinear approximation is obtained.

Immittance response of an electrolytic cell in the presence of adsorption, generation, and recombination of ions