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We report the magnetic structure of TaFe1+yTe3 single crystals by means ofneutron diffraction measurements. TaFe1+yTe3 possesses a layered structure witha formation of two-leg zigzag ladders along the b-axis. We find that TaFe1+yTe3undergoes an antiferromagnetic transition at 178 K with Fe1 spins of theintra-ladders ferromagnetically aligned while spins of the inter-laddersantiferromagneitcally coupled. Furthermore, spins of the neighboringinterstitial Fe2 (y) ions order parallel to the Fe1 spins of each ladder. Thesefindings are distinct from the magnetic structure of the recently-discoveredspin-ladder compound BaFe2Se3. TaFe1+yTe3 may serve as an interesting quasi-onedimensional ferromagnetic system.

Magnetic structure of quasi-1D antiferromagnetic TaFe1+yTe3 with two-leg zigzag ladders