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Combining macroscopic and diffraction methods we have studied the electric,magnetic and struc- tural properties of RE_(1-x)Ca_xTiO_3 (RE=Y, Er, Lu)focusing on the concentration range near the metal-insulator transition. Theinsulating phase, which is stabilized by a smaller rare-earth ionic ra- dius,exhibits charge order with a predominant occupation of the dxy orbital. Thecharge and orbital ordering explains the broad stability range of theinsulating state in RE_(1-x)Ca_xTiO_3 with smaller rare-earth ions. The strongmodulation of the Ti-O bond distances indicates sizeable modulation of theelectric charge.

Evidence for charge and orbital order in the doped titanates RE_(1-x)Ca_xTiO_3 (RE=Y, Er, Lu)