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Engineered nanoparticles made from noble metals, rare-earth oxides orsemiconductors are emerging as the central constituents of future nanotechdevelopments. In this review, a survey of the complexing strategies betweennanoparticles and oppositely charged polyelectrolytes developed during the lastthree years and based on electrostatic interactions is presented. Thesestrategies include the one-step synthesis of stable and functionalizednanoparticles, the one- and multilayer coating of individual nano-objects, thecontrolled clustering of particles and the generation of capsules and thinfilms with superior functionalities. Among the formulation processes reported,three main classes are identified : the direct mixing route, the desaltingtransition pathway and the well-known layer by layer method. Finally, somelatter developments, trends and applications of electrostatic assemblies inmaterials science and nanomedicine are highlighted

Versatile Electrostatic Assembly of Nanoparticles & Polyelectrolytes: Coating, Clustering and Layer-by-Layer Processes