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Pauling had proposed that charge is transferred from the more electronegativeatom to the less electronegative one during metallic alloying. An expressionhas recently been derived for the energy of the unlike atom-pair bond usingthat concept. In this paper, Pauling's view is further supported by showingthat the electronegativity and valence differences between unlike atoms inbinary metallic alloys are of the required magnitude and direction so as tobring the metallic radii ratio R_A/R_B by charge transfer to a value r_A/r_Bfor ideal packing in an intermetallic compound. It is also demonstrated thatlattice parameters of intermetallic compounds belonging to several crystalstructure types can be obtained with excellent accuracy from the length of theatom-pair bond.

Charge transfer on the metallic atom pair bond, and the crystal structures adopted by intermetallic compounds