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We propose a two-pulse excitation to efficiently photoinduced a novel$sp^3$-bonded nano-domain with a frozen shear in a graphite crystal. This$sp^3$ structure is known to be well stabilized by shear displacement betweenneighboring two graphite layers. This shear motion is generated only as atransient and unfrozen one by the first visible laser pulse, shone over thegraphite crystal. While, the second pulse is proved to freeze it before itdisappears, resulting in an efficient interlayer $\sigma$ ($sp^3$) bondformation.

Proposal of Two-Pulse Excitation to Efficiently Photoinduced Novel $sp^3$ Nano Domain with Frozen Shear in Graphite Crystal