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We present comprehensive molecular dynamics (MD) results for the kinetics ofsurface-directed spinodal decomposition (SDSD) and surface enrichment (SE) inbinary mixtures at wetting surfaces. We study the surface morphology and thegrowth dynamics of the wetting and enrichment layers. The growth law for thethickness of these layers shows a crossover from a diffusive regime to ahydrodynamic regime. We provide phenomenological arguments to understand thiscrossover.

Hydrodynamic Crossovers in Surface-Directed Spinodal Decomposition and Surface Enrichment