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Tailoring the phase stability and magnetic structure by combining theantiferromagnetic MnNiGe martensite with ferromagnetic MnFeGe austenite, amagnetic-field-induced martensitic transformation has been achieved inMnNi1-xFexGe system. The doped Fe enables the isolated structural and magnetictransitions of MnNiGe to coincide at room temperature and also establishesferromagnetic couplings in six-Mn-centering-one-Fe-atom clusters. Theferromagnetic clusters transit the antiferromagnetic state in martensite to aferromagnetic state and the alloys are further induced to a strongerferromagnetic state by external field, resulting in a large magnetizationdifference up to 50 emu/g across the transformation. The field-inducedmartensitic transformation thus experiences a multiple metamagnetizationprocess.

Field-induced multiple metamagnetization in phase transition from paramagnetic austenite to ferromagnetic martensite in MnNi1-xFexGe