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Reactions of hydrated halides​/perchlorate of cobalt(II)​, nickel(II) and copper(II) with 1,​2-​bis(N-​methylbenzimidazolyl)​benzene (L) in stoichiometric amts. in ethanol-​teof​/acetone​/thf produced complexes of the formulas MX2L·nH2O (n = 1, M = Co, X = Cl ; n = 0, M = Co, X = Br or I ; n = 0, M = Ni, X = I ; n = 0, M = Cu, X = Br)​, [MX2L (H2O)​] ( M = Ni, X = Cl or Br ; M = Cu, X = Cl)​, [Co(OClO3)​2(L)​1.5]​2·2H2O, [Ni(L)​2]​(ClO4)​2·H2O and [Cu(L)​2(OClO3)​]​ClO4·2H2O.  The complexes were characterised by elemental analyses, thermogravimetric anal., magnetic moment measurments, IR, electronic, NMR, ESR, mass spectral techniques.  Probable structures have been proposed for the complexes

Synthesis and spectral studies on Co (II), Ni(II) and Cu(II) complexes with 1,2- bis(N-methylbenzimidazolyl)benzene