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We have measured the magnetization of the organic compound BIP-BNO(3,5'-bis(N-tert-butylaminoxyl)-3',5-dibromobiphenyl) up to 76 T where themagnetization is saturated. The S = 1/2 antiferromagnetic Heisenberg two-legspin-ladder model accounts for the obtained experimental data regarding themagnetization curve, which is clarified using the quantum Monte Carlo method.The exchange constants on the rung and the side rail of the ladder areestimated to be J(rung)/kB = 65.7 K and J(leg)/kB = 14.1 K, respectively,deeply in the strong coupling region: J(rung)/J(leg) > 1.

Magnetization process of the S = 1/2 two-leg organic spin-ladder compound BIP-BNO