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Effects of coupling between a molecular exciton and a surface plasmon(exciton-plasmon coupling) on the luminescence properties of the molecule andthe surface plasmons are investigated using the nonequilibrium Green's functionmethod. Molecular absorption and enhancement by molecular electronic andvibrational modes (molecular modes) lead to dip and peak structures in theluminescence spectra of the surface plasmons. These structures will correspondto the peak and dip structures observed in a recent experiment. We found thatin addition to the molecular dynamics, the re-absorption by the surfaceplasmons plays important roles in determining the luminescence spectralprofiles.

Interplay between Plasmon Luminescence and Vibrationally Resolved Molecular Luminescence Induced by Scanning Tunneling Microscopy