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step in the biosynthesis of 1 is the formation of the precursor, 2-deoxy-scy//0-inosose (2), from D-glucose (3) via the intramolecular C-C bond formation between C-l and C-6.li2) The transformation of 3 into 2 was proposed by us to involve a multi-step mechanismas shownin Scheme1, the chemistry of which was suggested to be similar to the dehydroquinate synthase in the shikimate pathway,3'4* and an enzyme responsible of the intramolecular

journal of antibiotics

Biochemical studies on 2-deoxy-scyllo-inosose, an early intermediate in the biosynthesis of 2-deoxystreptamine. IV. A clue to the similarity of 2-deoxy-scyllo-inosose synthase to dehydroquinate synthase.