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The cri t ical temperatures, press ures, and vo lumes of H 2 , HD, and Dz have been determi ned by measurin g shor t sections of PF isotherms in t he neighborhood of t he cri t ical points. T he H 2 and Dz sa mples were ca taly zed to or tho-para equilibrium at 20.4° K and a re des ignated e-Hz a nd e-D.. Fo r e-Hz t he values found a re T , = 32.994 o K, P , = 12. 770 atm and 1', = 65. 5 cm3 mole-I. Fo r HD the corresponding values a re 35.908° K , 14.645 at m, and' 62.8 cm3 moleI; for e-Dz t he values a re 38. 26Zo K , 16. 282 atm, an cl 60. 3 cm3 m oleI. A m et hod of correlat in g isotherm data fo r different substances, based on t he use of g raphs of log P " ersus log Y, is described.

Critical temperatures, pressures, and volumes of hydrogen, deuterium, and hydrogen deuteride